Investigation of the photoionization process with zeptosecond precision

Entering the field of zeptosecond measurement

If light hits the two electrons of a helium atom, one must be incredibly fast to observe what occurs. Besides the ultra-short periods in which changes take place, quantum mechanics also comes into play. Laser physicists at the Max Planck Institute of Quantum Optics (MPQ), the Technical University of Munich (TUM) and the Ludwig Maximilians University (LMU) Munich have now measured such an event for the first time with zeptosecond precision.

Either the entire energy of a light particle (photon) can be absorbed by one of the electrons or a division  takes place, if a photon hits the two electrons of a helium atom. Regardless of the energy transfer, one electron leaves the atom. This process is called photoemission, or photoelectric effect, and was explained by Albert Einstein at the beginning of last century.

It takes between five and fifteen attoseconds (1 as is 10^-18 seconds) from the time a photon interacts with the electrons to the time one of the electrons leaves the atom, as physicists already discovered in recent years.

First glance into the world of Zeptoseconds

With their improved measurement method, laser physicists can accurately measure events at a rate of up to 850 zeptoseconds. The researchers shone an attosecond-long, extremely ultraviolet (XUV) light pulse onto a helium atom to excite the electrons.

At the same time, they fired a second infrared laser pulse, lasting about four femtoseconds (1 fs is 10^-15 seconds). The electron was detected by the infrared laser pulse as soon as it left the atom following excitation by XUV light.

Depending on the exact electromagnetic field of this pulse at the time of detection, the electron was accelerated or decelerated. Through this change in speed, the physicists were able to measure photoemission with zeptosecond precision.

In line with theoretical predictions

The researchers were also able to determine for the first time how the energy of the incident photon is quantum-mechanically divided between the two electrons of the helium atom in a few attoseconds before the emission of one of the particles.

"With the measurement of the electronic correlation, our experiments solved a promise of attosecond physics, namely the temporal resolution of a process which is inaccessible with other methods," says Reinhard Kienberger, professor of the Chair of Laser- and X-Ray Physics at TUM.

The physicists were also able to correlate the zeptosecond precision of their experiments with the theoretical predictions of their peers from the Institute of Theoretical Physics at the Technical University of Vienna.

Helium is the only multi electron system that can be calculated completely quantum mechanically. This makes it possible to reconcile theory and experiment. “We can now derive the complete wave mechanic description of the interconnected systems of electron and ionized helium mother atoms from our measurements,” says Martin Schultze, project leader at the Max Planck Institute of Quantum Optics in Garching (Germany).

With their metrology experiments in zeptosecond time dimensions, the laser physicists have maneuvered another important puzzle piece in the quantum mechanics of the helium atom into position, and thus advanced measuring accuracy in the microcosm to a whole new dimension.

The research was funded by the Max Planck Society, the German Research Foundation (DFG) via the Cluster of Excellence Munich-Center for Advanced Photonics (MAP), the Austrian Science Fund and the European Community (through two ERC grants and the Marie Curie program). In addition to the TU Munich and LMU Munich as well as the Max Planck Institute of Quantum Optics in Garching, the Technical University of Vienna and the Universidad Autónoma de Madrid participated in the project.

Publication:

M. Ossiander, F. Siegrist, V. Shirvanyan, R. Pazourek, A. Sommer, T. Latka, A. Guggenmos, S. Nagele, J. Feist, J. Burgdörfer, R. Kienberger and M. Schultze
Attosecond correlation dynamics
Nature physics, 7. November 2016, DOI: 10.1038/nphys3941

Contact:

Prof. Dr. Reinhard Kienberger
Technical University of Munich
Chair for Laser and X-ray Physics E11 and
Max Planck Institute of Quantum Optics
James Frank Str. 1, 85748 Garching, Germany
Tel.: +49 89 289 12840 - E-Mail - Internet